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    This dataset comprises calibrated geochemical data from stream sediment and soil samples collected in North Greenland between 1978 and 1999, supplemented by extensive reanalyses in 2011. The dataset includes selected elements relevant for the evaluation of zinc mineralisation: CaO, K₂O, Ba, Cu, Sr and Zn. A total of 2,469 stream sediment samples and 204 soil samples were included. The analytical values represent the most reliable results following systematic quality control and calibration procedures designed to eliminate bias between analytical methods and analytical periods, as described in Thrane et al. (2011). All values below detection limit are coded as 0 in the dataset. The dataset supports regional assessment of geochemical patterns and mineral potential in North Greenland.